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Cary /ˈkæri/ is the seventh-largest municipality in North Carolina. Cary is predominantly in Wake County, with a small area in Chatham County in the U.S. state of North Carolina and is the county's second-largest municipality and the third-largest municipality in The Triangle after Raleigh and Durham.The town's population was 135,234 as of the 2010 census (an increase of 43. % since 2000), making it the largest town and seventh-largest municipality statewide. As of April 2018, the town's estimated population was 162,025, though Cary was still considered a town because that is how it was registered with the state. Cary is the second most populous incorporated town (behind only Gilbert, Arizona) in the United States.